Section 1:

Introduction

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Introduction

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      The main goal of this paper is to introduce and describe five species of minerals which are represented in a small collection brought out of the copper mines of Butte, Montana during the 1950's. The species included in the collection are native copper, azurite, malachite, rhodocrosite, and chrysocolla. Their description is contained in Section 6, which is the final portion of the paper.
      Section 6 states the species and class of the five minerals represented in the collection. It then describes the physical characteristics of these species. It discusses their color, mentions their streak, luster, density, and hardness, and notes characteristic patterns of cleavage and fracture. It relates their crystal class, and states their crystal habit and preferred patterns of crystalline growth. Finally it mentions in what type of environment and in the company of which other species these minerals may be found.
      Sections 1 through 5 attempt to explain the terminology and ideas which are utilized in Section 6 to describe the minerals of the collection. In Section 1 the paper first attempts to define the set of characteristics which cause certain crystalline natural substances to be defined as minerals. In Section 2 it continues with a description of the physical attributes of minerals. These attributes include such characteristics as color, luster, density, hardness, and preferred patterns of crystal growth. Section 3 then considers the structure, symmetry and shapes which may be possessed by crystals. It introduces the six systems and thirty-two classes into which crystals are categorized on the basis of their symmetry features. The fourth section of the paper explains the system of classification under which each mineral species is assigned to a particular mineral class according to certain chemical criteria. Section 5 explains the different geologic processes by which rocks and minerals are formed. Section 6 finally utilizes the information presented in the first five sections in order to describe the five mineral species represented in the small collection.


Definition of a Mineral

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      A mineral is defined to be a naturally occurring, homogeneous crystalline solid. A mineral must first of all be a solid; this requirement excludes all liquids and gases. A crystalline material is not merely a solid but also possesses an orderly and periodic molecular structure. This molecular structure is composed of repeated units, each of which contains a specified set of atoms or ions placed according to a specified geometric arrangement. The periodic repetition of such unit cells results in discrete translational invariance within the crystal lattice. An amorphous solid such as amber, coal, or glass does not possess this orderly, periodic, translationally invariant crystalline lattice structure and thus may not be considered a mineral.
      Minerals are expected to be homogeneous: the chemical composition of a mineral may not differ significantly from sample to sample within a species or from location to location within a sample. However, small variations in chemical composition are permissable. In certain species the chemical composition may vary over a well-defined range. Two samples, each of which possesses a chemical composition which falls within the required range, are then considered to be minerals of the same species despite any difference in their compositions. Trace amounts of impurities, or elements which are not an integral part of the crystal structure, may also be present within the crystal lattice. The atoms of an impurity may either occupy a previously uninhabited position within a few individual unit cells or they may replace a few atoms which are regularly part of the lattice. Such impurities may not be present in large quantities and they may not greatly affect any physical properties of the mineral species except color, hardness, and conductivity.
      The requirement that a mineral be naturally occurring was conceived before the production of synthetic materials was prevalent. In recent years, however, a multitude of synthetic materials which would otherwise satisfy the definition of a mineral have been produced in the laboratory. These substances are rapidly gaining in importance in both industry and experiment, and it now seems logical to extend the definition of 'mineral' in order to include such synthetic materials.


The Physical Characteristics of Minerals

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      The physical properties of a mineral are determined by its chemical composition and its crystalline structure. Within the limits of the permissible variation in chemical composition, different samples of a single mineral species are expected to display the same set of physical properties. These characteristic physical properties are therefore very useful to the field geologist in identifying and describing a specimen.
      Properties which describe the physical appearance of a mineral specimen include color, streak, and luster. Mass-dependent properties include density; mechanical properties include hardness, cleavage, fracture, and tenacity. Properties relating to the growth patterns and physical appearance of crystals, both individually and in aggregate, are described in terms of crystal habit, crystal form, and crystal system.
      Some minerals derive their color from the presence of an element which is defined to be part of the crystal lattice. Coloration of this type is termed allochromatic coloration. Different samples of a mineral species which possesses allochromatic coloration will all display the same color. Other minerals are colored by the presence of certain elements in mixture. These minerals may exhibit a range of colors. Still other mineral species may usually be colorless, but may display several startling and different colors when trace amounts of impurities are present. This type of coloration is termed idiochromatism. Certain elements are strong pigmenting agents and may lend vivid colors to specimens when they are present, whether as a part of the crystal lattice, in mixture, or as an impurity. Such elements are called chromophores. The color which a mineral displays when it has been ground to a fine powder is termed streak. Trace amounts of impurities do not tend to affect the steak of a mineral, so this characteristic is usually more predictable than color.
      Minerals are either opaque or transparent. A thin section of an opaque mineral will not transmit light, whereas a thin section of a transparent mineral will. Relative differences in opacity and transparency are described as luster. The characteristic of luster refers to the amount and quality of light which is reflected from a mineral's exterior surfaces, and provides a description of how much the mineral surface 'sparkles'.
      The property of density is defined as mass per unit volume. Hardness is defined as the amount of difficulty with which a mineral specimen may be scratched. Hardness has traditionally been measured according to the Mohs scale, but the diamond indentation method now provides a more quantitative measurement. The cleavage of a crystal refers to its propensity for splitting along a smooth plane. A cleavage plane is a plane of structural weakness. The property which is termed cleavage refers to both the ease with which the mineral cleaves and to the character of the exposed surface. Not every mineral exhibits cleavage. Fracture takes place when a mineral sample is split in a direction which does not serve as a plane of cleavage. A mineral fractures when it is broken or crushed. In some mineral species fractured surfaces may possess a characteristic appearance.
      The term crystal habit describes the favored growth pattern of the crystals of a mineral species. The crystals of particular species sometimes form very distinctive, characteristic shapes. Crystal habit is also greatly determined by the environmental conditions under which a crystal develops.


The Classification of Crystals

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      The descriptive terminology of the discipline of crystallography is applied to crystals in order to describe their structure, symmetry, and shape. This terminology describes the crystal lattice, which provides a mineral with its ordered internal structure. It also describes and analyzes various types of symmetry. By considering what type of symmetry a mineral species possesses, the species may be categorized as a member of one of six crystal systems and one of thirty-two crystal classes.
      The concept of symmetry describes the periodic repetition of structural features. Two general types of symmetry exist. These include translational symmetry and point symmetry. Translational symmetry describes the periodic repetition of a motif across a length or through an area or volume. Point symmetry, on the other hand, describes the periodic repetition of a motif about a single point. Reflection, rotation, inversion, and rotoinversion are all point symmetry operations.
      A specified motif which is translated linearly and repeated many times will produce a lattice. A lattice is an array of points which define a repeated spatial entity called a unit cell. The unit cell of a lattice is the smallest unit which can be repeated in three dimensions in order to construct the lattice.
      The number of possible lattices is limited. In the plane only five different lattices may be produced by translation. The French crystallographer Auguste Bravais (1811-1863) established that in three-dimensional space only fourteen different lattices may be constructed. These fourteen different lattices are thus termed the Bravais lattices.
      The reflection, rotation, inversion, and rotoinversion symmetry operations may be combined in a variety of different ways. There are thirty-two possible unique combinations of symmetry operations. Minerals possessing the different combinations are therefore categorized as members of thirty-two crystal classes. In this classificatory scheme each crystal class corresponds to a unique set of symmetry operations. Each of the crystal classes is named according to the variant of a crystal form which it displays. Each crystal class is grouped as one of the six different crystal systems according to which characteristic symmetry operation it possesses.
      A crystal form is a set of planar faces which are geometrically equivalent and whose spatial positions are related to one another by a specified set of symmetry operations. If one face of a crystal form is defined, the specified set of point symmetry operations will determine all of the other faces of the crystal form. A simple crystal may consist of only a single crystal form. A more complicated crystal may be a combination of several different forms. Example crystal forms are the parallelohedron, prism, pyramid, trapezohedron, rhombohedron and tetrahedron.
      Each crystal class is a member of one of six crystal systems. These include the isometric, hexagonal, tetragonal, orthorhombic, monoclinic, and triclinic crystal systems. Every crystal of a certain crystal system shares a characteristic symmetry element - for example, a certain axis of rotational symmetry - with the other members of its system. The crystal system of a mineral species may sometimes be determined by examining a particularly well-formed crystal of the species.


Mineral Classification

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      The Berzelian mineral classification system was named in honor of the Swedish chemist and mineralogist Jons Jakob Berzelius (1779-1848). The Berzelian system categorizes mineral species according to the main anion group present in their chemical composition. Mineral classes may then be further subdivided according to physical features, the presence of certain cations in the lattice, the presence or absence of water or the hydroxyl anion, or structural considerations. The main classes which are recognized under Berzelius' scheme include the native elements; sulfides and sulfosalts; oxides and hydroxides; halides; carbonates, nitrates and borates; sulfates; phosphates; and silicates. The antimonides, arsenides, selenides, and tellurides closely resemble the sulfides, while the chromates, molybdates and tungstates resemble the sulfates. The arsenates and vanadates are closely akin to the phosphates.
      The native elements include all mineral species which are composed entirely of atoms in an uncombined state. Such minerals either contain the atoms of only one element or else are metal alloys. The native elements are divided into metallic, semimetallic, and nonmetallic subgroups. Metals tend to be dense and malleable substances which possess a characteristic metallic luster and conduct electricity well, while semimetals and nonmetals tend to be brittle and to conduct poorly.
      Minerals of the sulfide class are compounds which contain the nonmetallic element sulfur in combination with atoms of a metal or a semimetal. Compounds in which anions of antimony (Sb), arsenic (As), selenium (Se), or tellurium (Te) replace the sulfur anion and bond with metallic or semimetallic cations are classed respectively as antimonides, arsenides, selenides, and tellurides. If the sulfur anion, a metallic element, and a semimetal are all present then the mineral is categorized as one of the rare sulfosalts. Most sulfides and sulfosalts are soft, dark, heavy, and brittle, possessing a metallic luster and high conductivity.
      The minerals of the oxide class contain oxygen bonded to one or more metallic elements. Hydroxides are compounds of a metallic element and water or the hydroxyl anion (OH-). The oxide minerals tend to be relatively hard. Many provide important metal ores, and some of them may be used as gemstones. Minerals of the hydroxide class tend to be softer and less dense than oxides.
      In members of the halide class an element of the halogen group such as fluorine (F), chlorine (Cl), bromine (Br), or iodine (I) bonds to a metal or semimetal cation such as sodium (Na), potassium (K), magnesium (Mg), calcium (Ca), aluminum (Al), copper (Cu), or silver (Ag). Halides are constructed entirely of ionic bonds. The halides tend to be soft, brittle, easily soluble in water, and possess medium to high melting points. In solid state they are poor conductors.
      Mineral species which are members of the carbonate class are compounds of a metal or semimetal with the carbonate anion (CO3)2-. The nitrates are structurally very closely akin to the carbonates with the nitrate anion (NO3)- replacing the carbonate anion. The nitrates tend to be softer and to possess lower melting points than do the carbonates. Minerals of the borate class contain the borate radical (BO3)3- rather than the carbonate or nitrate radicals. However, borate radicals may unlike the carbonate or nitrate radicals be linked into polymerized chains, sheets, or groups. This trait grants the minerals of the borate class unique structural characteristics.
      This sulfate radical (SO4)2- forms the basic structural unit of the minerals of the sulfate class. Minerals of the chromate class are compounds of metallic cations with the chromate anion group (CrO4)2-. Just as sulfur and chromium form the anion groups (SO4)2- and (CrO4)2-, the ions of molybdenum (Mo) and tungsten (W) bond with oxygen atoms to create the anion groups (MoO4)2- and (WO4)2-. These anion groups then bond with metal cations to form the minerals of the molybdate and tungstate classes.
      Like sulfur, the elements phosphorous (P), arsenic (As), and vanadium (V) form anion groups in combination with oxygen. The resulting phosphate radical, (PO4)3-, provides the basic structural unit of the minerals of the phosphate class; the arsenate and vanadate radicals (AsO4)3- and (VaO4)3- form the basic structural units of the arsenate and vanadate classes. The mineral species of these three classes are thus composed of the respective phosphate, arsenate, and vanadate radicals linked by various metal and semimetal cations.
      The basic constituent of the minerals of the silicate class is the silicate radical (SiO4)4-. Silicate radicals may remain structurally isolate, join together in pairs, or polymerize into frameworks, sheets, chains, or rings. The various species of the silicate class are grouped according to their structural type. Silicate minerals are usually of relatively great hardness, and single crystals are often translucent.


Petrogenesis

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      The term petrogenesis refers to the means by which a rock or mineral deposit is formed. Three different modes of formation are common; these consist of igneous activity, metamorphism, and sedimentary processes. Mineral deposits therefore occur in these three types of environments and also in vein environments.
      Igneous rocks are formed when magma or molten rock cools and solidifies. Some igneous rocks form from magma which cooled at great depths within the earth's crust, while others formed when magma erupted from a volcano or vent at the earth's surface. Metamorphism describes the set of solid state processes which transform one type of rock into another. Any type of rock, whether igneous, metamorphic, or sedimentary, may be metamorphised. Metamorphism typically occurs at the high temperatures and pressures found deep within earth's crust. Veins are mineral deposits which form when a fracture or fissure within a larger body of rock is filled with new crystalline material. Veins are believed to form when aqueous solutions migrate through fissures in rock and deposit minerals onto the fissure walls. Sedimentary rock is formed when loose sediments are collected together, compacted, and cemented into rock through the action of heat, pressure, and chemical agents. These sediments may be derived from the erosion of preexisting rocks, by precipitation from aqueous solution, or from the skeletal remains of organisms. They are transported and collected via meteorological processes such as flowing water, wind, and migrating glaciers.


Specimens of the Collection

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Photos of the collection

      The small collection of minerals with which this paper is concerned contains five species. All samples in the collection were removed from the copper mines of Butte, Montanna during the 1950's. Native copper, the copper carbonates azurite and malachite, and the amorphous copper silicate chrysocolla are copper-bearing substances. Rhodocrosite (MnCO2) is, like azurite and malachite, a carbonate mineral, but is an ore of manganese rather than a copper ore.
      Copper (Cu) is a native metal which has long been utilized as a resource by humans. It is composed of only elemental copper and its physical features are derived from the prevalent metallic bonds of its structure. Like all metals, native copper is dense, soft, malleable, and ductile; it conducts well. It is opaque and possesses the shiny, highly reflective luster typical of metals. In color it is the familiar, rosy copper red; it possesses a red streak. Native copper demonstrates a face-centered cubic lattice, which is the most dense and symmetric of all possible crystalline structures. It is of the isometric or cubic crystal system. Individual copper crystals may may be of cubic, dodecahedral, tetrahedral, and very rarely of octahedral shape. Aggregates of crystals may be wiry in habit or form a dendritic, arborescent branching structure.
      The two minerals azurite (Cu3(CO3)2(OH)2) and malachite (Cu2Co3(OH)2) are closely related. Both are hydrous copper carbonates. Azurite is royal blue or brilliant blue in color while malachite may be bright to dark green. The coloration in both species is idiochromatic and is due to the presence of the chromophore copper, which has a strong pigmenting effect. Aggregates of crystals of both species are frequently botryoidal or mammillary in habit. Large individual crystals of malachite are rare. More commonly the mineral occurs in rings, bands, and concentric layers of varying shades of green. Both azurite and malachite occur as earthy, incrusted masses.
      Rhodocrosite (MnCO3) is member of the carbonate class, a member of calcite group, and an ore of manganese. Its characteristic rose pink or red color is idiochromatic and is due to the presence of the chromophore manganese (Mn). Rhodocrosite is translucent and will transmit light diffusely; it possesses a vitreous or pearly luster.
      Rhodocrosite is like all calcite minerals a member of the rhombohedral crystal system. Rhodocrosite's cleavage is perfect in three directions and is rhombohedral. Crystals are rare but may be rhombohedral in shape; more typically the mineral demonstrates botryoidal, encrusting habit.
      The hydrous silicate chrysocolla (Cu2H2Si2O5(OH)4) is an ore of copper. Chrysocolla is not a true mineral and does not possess a crystalline lattice. Instead, it is an amorphous 'silica gel' or gelatinous precipitate. It is, however, a copper-bearing solid substance and is commonly found in association with minerals such as azurite, malachite, and native copper. Chrysocolla is green to sky-blue in color. This coloration is idiochromatic and is due to the presence of the chromophore copper (Cu). Chrysocolla is translucent; samples may be of vitreous or glassy luster or appear greasy, dull, or earthy. It has no cleavage and demonstrates uneven or conchoidal fracture. Specimens of chrysocolla are typically of massive or earthy habit. The substance may also display reniform or bulbous, botryoidal habit.
      Azurite, malachite and chrysocolla are commonly found in the oxidized zones of copper veins and deposits. Rhodocrosite occurs in veins and hydrothermal replacement deposits in the company of manganese minerals as well as other metal ores such as copper.


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